2D titanium carbide (MXene) electrodes with lower-F surface for high performance lithium-ion batteri

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MXene has shown distinctive advantages as anode materials of lithium-ion batteries.However,local surface chemistry,which was confirmed that can block ion transfer and limit redox reaction,has a significant effect on electrochemical performance.Herein,annealing MXene under hydrogen was employed for removing-F and turning-OH to-O terminations.We demonstrate that it improves the kinetics of Li-ion transport between the electrolyte and electrode.As a result,a lower interfacial charge transfer impedance was obtained.The electrochemical measurement exhibited that a nearly 2-fold increase of specific capacity was achieved for the annealed MXene.
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