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A new compound K_6Ti_2Nb_(14)O_(42)was found inthe ternary system K_2O-TiO_2-Nb_2O_5.The compound was char-acterized and investigated by electron,probe,X-ray powderdiffraction and differential thermal analysis.The transpar-ent crystal of light yellow color in form of hexagon-thinplate can be grown by flux method.Further,its crystal struc-ture was determined by four-circle diffratometer K_6Ti_2Nb_(14)O_(42)crystallizes in he(?)(?)(?)onal system with unitcell parameters a=9.1106(5)×10~(-10)m·c=12.0136(9)×10~(-10)m,Z=l andspace.group P6_3/mcm(193).