,Temperature dependent terahertz giant anisotropy and cycloidal spin wave modes in BiFeO3 single cry

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THz time-domain spectroscopy (THz-TDS) is used to study the THz-optical properties of a single crystal bismuth ferrite BiFeO3 (BFO).It can be found that the anisotropy of BiFeO3 is strongly dependent on the temperature.A giant birefringence up to around 3.6 is observed at 1 THz.The presence of a spatially modulated cycloidal antiferromagnetic structure leads to spin cycloid resonances (SCR) φ and φ,corresponding to the out-of-plane and in-plane modes of the spin cycloid,respectively.We distinguish the SCR with respect to their response to orthogonal polarizations of the electric fields of the incident THz beam.In addition,we observe a resonance appearing below 140 K,which might be interpreted as an electromagnon mode and related to a spin reorientation transition.Our present observations present that the temperature and polarization,as the exteal control parameters,can be used to modulate the THz optical properties of BFO single crystal.
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