Fe-based phosphate nanostructures for supercapacitors

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Fe-based phosphates with excellent physical and chemical features are potential electrode materials for supercapacitors.In this work,we successfully synthesized Fe-based phosphates with different dimensions,morphologies,and compositions by one-step hydrothermal method.Influence factors on the chemical composition and morphology of the as-prepared materials were explored and the energy storage performance of the as-prepared samples were tested under the traditional three electrode system.Two-dimensional (2D) iron metaphosphate (Fe(PO3)3) showed the best electrochemical performance.For Fe(PO3)3 electrode materials,the layered structure can provide a larger specific surface area than the bulk structure,which is conducive to the diffusion and transport of electrolyte ions during charging-discharging and further improves the rate performance and cycle stability of supercapacitor.2D Fe(PO3)3 and activated carbon were used as electrode materials to construct a 2D Fe(PO3)3//AC supercapacitor.The supercapacitor showed high energy density,high power density,and excellent cycling stability,which indicates 2D Fe(PO3)3 is a promising electrode material for supercapacitors.
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