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We present experimental measurements that show direct determination of the dielectric properties of various metals relevant to plasmonics. In contrast to traditional measurements that typically rely on transmission and reflectance measurements, we launch surface plasmon-polaritons on a variety of different substrates and measure the propagation properties using terahertz time-domain spectroscopy. Surprisingly, we find that the extracted values for the dielectric constant for these metals differ by orders of magnitude from published data. In order to validate the obtained results, we separately measure the 1∕e decay length, both along the propagation direction and normal to the metal surface, and show that the results are fully self-consistent with experimental data. The generality of the measurement technique makes it a useful tool to estimate the properties not only of planar conducting substrates but also a wide variety of more complex plasmonic structures.