【摘 要】
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The response theory is used to investigate one-and two-photon absorption (TPA) as well as emission properties of a series of potential zinc ion and pH sensitive
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The response theory is used to investigate one-and two-photon absorption (TPA) as well as emission properties of a series of potential zinc ion and pH sensitive materials containing 2-(2’-hydroxyphenyl)benzoxazole (HPBO) end groups. Special emphasis is placed on the evolution of their optical properties upon combining with zinc ions or deprotonation. Calculated results indicate that upon combining with zinc ions or deprotonation, these HPBO derivatives show drastic changes in their one-photon absorption (OPA), emission, and TPA properties. Moreover, mechanisms of the probes are analyzed to be intramolecular charge transfer. These compounds are thus proved to be excellent candidates for two-photon fl uorescent zinc and pH probes.
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