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In this paper,[1] we report two novel D-pi-D hole-transporting materials(HTM),abbreviated as BDT-PTZ and BDT-POZ,which consists of 4,8-di(hexylthio)-benzo[1,2-b:4,5-b]dithiophene(BDT)as conjugated linker,and N-(6-bromohexyl)phenothiazine(PTZ)/N-(6-bromohexyl)phenoxazine(POZ)as donor units.